At the moment, if you’re looking to play games on Chrome OS, you’re more or less limited to finding those games on the Google Play Store. That may all be changing at some point in the near future, as Google has suggested that it’s working with Valve to build official Steam support for Chrome OS. This, of course, would greatly expand the gaming capabilities of Chromebooks by allowing them to tap into Steam’s vast library of PC titles.
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https://www.slashgear.com/chrome-os-may-finally-get-official-steam-support-17607059/